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Kurosaki, Yuzuru*; Yokoyama, Keiichi
Chemical Physics, 493, p.183 - 193, 2017/08
Times Cited Count:5 Percentile:21.67(Chemistry, Physical)Electric field of laser pulses which gives maximum selectivity in the isotope-selective rovibrational excitation of lithium chloride molecules is calculated. Applying the optimal control theory, we calculate optimal electric field to produce mixture of LiCl-35 (=0, =0) and LiCl-37 (=1, =1) from molecular ensemble of LiCl-35 (=0, =0) and LiCl-37 (=0, =0). As a result, it is found that electric field which permit rotational excitations only gives high yield in the selective excitation compared to the electric field which permit both rotational and vibrational excitations.
Ichikawa, Shoichi; Chiba, Yusuke; Ono, Fumiyasu; Hatori, Masakazu; Kobayashi, Takanori; Uekura, Ryoichi; Hashiri, Nobuo*; Inuzuka, Taisuke*; Kitano, Hiroshi*; Abe, Hisashi*
JAEA-Research 2017-001, 40 Pages, 2017/03
In order to reduce the influence on a plant schedule of the MONJU by the maintenance of dew point hygrometers, The JAEA examined a capacitance type dew point hygrometer as an alternative dew point hygrometer for a lithium-chloride type dew point hygrometer which had been used at the CV-LRT in the MONJU. As a result of comparing a capacitance type dew point hygrometer with a lithium-chloride type dew point hygrometer at the CV-LRT (Atmosphere: nitrogen, Testing time: 24 hours), there weren't significant difference between a capacitance type dew point hygrometer and a lithium-chloride type dew point hygrometer. As a result of comparing a capacitance dew point hygrometer with a high-mirror-surface type dew point hygrometer for long term verification (Atmosphere: air, Testing time: 24 months), the JAEA confirmed that a capacitance type dew point hygrometer satisfied the instrument specification (2.04C) required by the JEAC4203-2008.
Kurosaki, Yuzuru*; Yokoyama, Keiichi
no journal, ,
Electric field of laser pulses is designed by the optimal control theory. The target process is isotope-selective rovibrational excitation of two isotopologues of the lithium chloride molecule, LiCl or LiCl. The calculation includes both radial and angular motion of atoms in molecule. As a result, it is found that a laser pulse field which can cause isotope-selective rovibrational excitation with high yield exists.